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DBD等离子体处理火驱尾气中稀薄甲烷的实验研究

Experimental Study on the Treatment of Lean Methane in Fire-Flooding Tail Gas by DBD Plasma

  • 摘要: 本文采用了介质阻挡放电非平衡态等离子体技术对火驱尾气中稀薄甲烷进行低温高效处理。实验考察了等离子体放电功率(21~46 W),O2/CH4摩尔比(2~10)和气体流量(400~1200 mL/min)对CH4转化率、CO2和CO选择性的影响。结果表明,随着放电功率和O2/CH4摩尔比的增加以及气体流量的降低,CH4的转化率提高,CO2和CO的选择性分别呈上升和下降的趋势。在高的放电功率和O2/CH4摩尔比、低的气体流量的条件下可实现稀薄甲烷的完全转化;稀薄甲烷氧化基本以生成CO为主,其次是CO2,CO的选择性最高可达98.89%,CO2的约为56.63%。

     

    Abstract: In this paper, dielectric barrier discharge non-equilibrium plasma technology is used to treat lean methane in the exhaust gas of fire flooding. The effects of plasma discharge power (21~46 W), O2/CH4 molar ratio (2~10), and gas volume flow rate (400~1200 mL/min) on CH4 conversion rate, CO2 and CO selectivity were investigated. The results show that with the increase of discharge power and O2/CH4 molar ratio, as well as the decrease of gas flow rate, the conversion rate of CH4 increases, and the selectivity of CO2 and CO shows an upward and downward trend, respectively. Under the condition of high discharge power and O2/CH4 molar ratio, and low gas flow rate, complete conversion of lean methane can be achieved. The oxidation of lean methane mainly produces CO, followed by CO2. The selectivity of CO can reach up to 98.89%, while that of CO2 is about 56.63%.

     

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