Experimental Study on the Treatment of Lean Methane in Fire-Flooding Tail Gas by DBD Plasma
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Graphical Abstract
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Abstract
In this paper, dielectric barrier discharge non-equilibrium plasma technology is used to treat lean methane in the exhaust gas of fire flooding. The effects of plasma discharge power (21~46 W), O2/CH4 molar ratio (2~10), and gas volume flow rate (400~1200 mL/min) on CH4 conversion rate, CO2 and CO selectivity were investigated. The results show that with the increase of discharge power and O2/CH4 molar ratio, as well as the decrease of gas flow rate, the conversion rate of CH4 increases, and the selectivity of CO2 and CO shows an upward and downward trend, respectively. Under the condition of high discharge power and O2/CH4 molar ratio, and low gas flow rate, complete conversion of lean methane can be achieved. The oxidation of lean methane mainly produces CO, followed by CO2. The selectivity of CO can reach up to 98.89%, while that of CO2 is about 56.63%.
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